Novel Functional Materials Based on Polymer-Polyoxometallete Hybrids

Wei WANG

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Novel Functional Materials Based on Polymer-Polyoxometallete Hybrids

更新时间：2022-09-18

- Novel Functional Materials Based on Polymer-Polyoxometallete Hybrids
- Polymer Bulletin Vol. 26, Issue 1, Pages: 87-100(2013)
- 作者机构：
  
  南开大学功能高分子教育部重点实验室和高分子研究所，合成软材料中心，天津　300071
- 作者简介：
- 基金信息：
- DOI：
  CLC：
- Published：2013-01，
  
  Received：28 August 2012，
  
  Revised：12 September 2012，
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Wei WANG. Novel Functional Materials Based on Polymer-Polyoxometallete Hybrids. [J]. Polymer Bulletin 26(1):87-100(2013)
DOI：

Wei WANG. Novel Functional Materials Based on Polymer-Polyoxometallete Hybrids. [J]. Polymer Bulletin 26(1):87-100(2013) DOI：

摘要

随着学科之间相互交叉渗透的发展

兼有无机材料的功能性和有机材料的可加工型的新型杂化材料显示出了巨大的应用前景。本篇论述介绍本研究组在过去几年里

将多金属氧酸盐簇(Polyoxometalates)与我们熟知的聚合物通过共价键相连接制备杂化物(Polyoxometalate-Polymer Hybrids

PPHs)的研究结果

目的是在保证POMs簇合物特殊功能的前提下

还赋予杂化物良好的可加工性能

开发高附加值的功能杂化材料。通过对含PPHs的合成和超分子聚集体自组装行为的研究工作

将POMs簇合物化学、聚合物化学和超分子科学的相关知识融合在一起

并在这三个传统研究方向的交叉点上开辟了一个新的突破领域

该研究成果为先进功能材料的制备提供了一个新的思路。

Abstract

In this account

we repoted our efforts in the development of polyoxometalate-polymer hybrids (PPHs) using new polymerization methods. It is worthy to point out that the polyoxometalate clusters are covalently linked with polymers in the PPHs. Our target is to prepare a high value-added PPH materials with functionalities of polyoxometalates and processability of polymers. In our work we have desgined and sythesized two kinds of PPHs using atom transfer radical polymerization (ATRP) and clicking reaction

respectively. Meanwhile we studied the self-assembled structures and morphologies of the PPHs that strongly affected by the special architecture of polyoxometalates. This work reflects an interdiscipline of polyoxometalate chemistry

polymer chemistry and supramolecular self-assembly. Our findings will provide a new pastway in creating novel functional materials.

关键词

杂化材料聚合物多金属氧酸盐簇

Keywords

Hybrid materialsPolymersPolyoxometallets

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