Upgrading Waste Poly(ethylene terephthalate) into Carbon Material and Metal-Organic Framework

FAN Zi-fen; LIU Hua-jian; LIU Li-jie; NIU Ran; LIU Jie; GONG Jiang

doi:10.14028/j.cnki.1003-3726.2023.11.006

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Upgrading Waste Poly(ethylene terephthalate) into Carbon Material and Metal-Organic Framework

Special Issue: Polymer Research at Huazhong University of Science and Technology | 更新时间：2023-10-12

- Upgrading Waste Poly(ethylene terephthalate) into Carbon Material and Metal-Organic Framework
- Polymer Bulletin Vol. 36, Issue 11, Pages: 1454-1470(2023)
- 作者机构：
  
  1.能量转换与存储材料化学教育部重点实验室，材料化学与服役失效湖北省重点实验室，华中科技大学化学与化工学院，武汉　430074
  2.湖北大学材料科学与工程学院，武汉　430062
- 作者简介：
- 基金信息：
- DOI：10.14028/j.cnki.1003-3726.2023.11.006
  CLC：
- Published：20 November 2023，
  
  Received：03 June 2023，
  
  Revised：21 June 2023，
扫描看全文
FAN Zi-fen, LIU Hua-jian, LIU Li-jie, NIU Ran, LIU Jie, GONG Jiang. Upgrading Waste Poly(ethylene terephthalate) into Carbon Material and Metal-Organic Framework. [J]. Polymer Bulletin 36(11):1454-1470(2023)
DOI：

FAN Zi-fen, LIU Hua-jian, LIU Li-jie, NIU Ran, LIU Jie, GONG Jiang. Upgrading Waste Poly(ethylene terephthalate) into Carbon Material and Metal-Organic Framework. [J]. Polymer Bulletin 36(11):1454-1470(2023) DOI： 10.14028/j.cnki.1003-3726.2023.11.006.

摘要

伴随着聚对苯二甲酸乙二醇酯(PET)被广泛应用于饮料瓶、纺织、薄膜和合成纤维，大量废弃 PET 制品造成的环境污染问题日益突出。将废弃PET升级化学回收，制备高附加值产品是解决废弃PET 环境污染问题及使资源可持续发展的重要技术。结合本研究组在该领域的工作，本文介绍了近年来废弃 PET高值化制备多孔碳和金属-有机框架材料(MOF)的研究进展，归纳了不同类型多孔碳和MOF的制备方法，总结了PET 降解和碳化反应的影响因素和反应机理，概述了所制备的多孔碳和MOF在太阳能界面水蒸发以及与光催化降解污染物、热电发电集成中的应用，对未来的发展方向进行了展望。

Abstract

With the widespread application of poly(ethylene terephthalate) (PET) in beverage bottles

textiles

film

and synthetic fibers

the environmental pollution caused by discarded PET products is becoming increasingly prominent. Chemical upcycling of waste PET to prepare high value-added materials is an important technology to solve the environmental pollution problem of waste PET and ensure sustainable development of resources. Based on the work of our research group in this field

this article introduces the research progress on the preparation of high-value porous carbon and metal-organic framework (MOF) material from waste PET in recent years

summarizes the preparation methods of different types of porous carbon and MOF

introduces the influencing factors and reaction mechanisms of PET degradation and carbonization reaction

and discusses the applications of the prepared porous carbon and MOF in interfacial solar-driven water evaporation and its integration with photocatalytic degradation of pollutants and thermoelectric power generation. Prospects are made for the future development direction.

关键词

聚对苯二甲酸乙二醇酯碳材料金属-有机框架材料太阳能界面水蒸发

Keywords

Poly(ethylene terephthalate)Carbon materialMetal-organic framework materialInterfacial solardriven water evaporation

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能量转换与存储材料化学教育部重点实验室，材料化学与服役失效湖北省重点实验室，华中科技大学化学与化工学院

湖北大学材料科学与工程学院

Laboratory of Polymer Physics and Chemistry, Institute of Chemistry, Chinese Academy of Sciences

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